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He called this connection the equivalence principle. inheritance. Youre free to do whatever you want with them, 166±167 Cope rearrangement, 164, 166 component analysis, 168 Silaethene p bond energy, 104 Silaethenes, 103±104 Silane reaction with silyl radical, 149 reaction with thiyl radical, 149 Silyl cations, 108 Silyl radical reaction with silane, 149 Silylenes, 116 Simple HuÈckel molecular orbital theory, 86±97 alpha, 87 approximations, 87 beta, 87 Slater determinant, 251, see also Determinantal wave function SN1 mechanism, 129±130 alkyl halides, 129 carbocation intermediates in, 106 leaving group, 130 Lewis acid catalysis, 130 SN2 mechanism, 130±136 alkyl halides, 130 carbocation intermediates in, 106 and E2, 143 gas phase, 144 geometry of approach, 131 leaving group, 130, 132 nucleophilicity, 131±132 substituent e ̈ects, 132±134 transition state, 132, 133 VBCM description, 134±135 Snoutene, 247 rearrangement, 289 Sodium borohydride, 83, 278 Sodium hydride, 83 Soft Electrophiles, 110 reaction with enolate, 110 Spin function, 234 Spin-Spin Coupling, and ss character, 16 Spiropentadiene, 273 Split valence basis set, 24±25 State correlation diagrams, 203±208 carbene to alkene, 207 Dauben±Salem±Turro, 212±213 Norrish type I, 215±217 Norrish type II, 213±215 from orbital correlation, 203±206 rules for, 206 Stationary point, 209 Steric interaction, 47 Stereoisomers, 8 Stereoheterotopic groups, 9 STO-nG, 24 Structures of ®rst row hydrides, 32 Styrene SHMO, 153 Substituent types, 99 see C'' substituents see X: substituents see Z substituents Sudden polarization, 272 a-Sulfonyl carbanion, 277±278 Sulfuric acid, 100 Suprafacial, 163 examples, 164 sigma bonds, 167 Synthesis, asymmetric, de®nition, 9 Tachysterol3, 310 Tetracoordinated metals FeCl4, 184 Fe(CO)4, 184 Ni(CO)4, 184 orbitals of, 182±184 Tetracyanoethylene, 273 Tetrahydrofuran BF3 a12nity, 123 IP, 123 PA, 123 Tetramesityldisilene, 104 Tetramethylcyclobutadiene, 296 Tetrazenes, 118 Thiirane, 253 cation, 253 Thiiranes ring opening, 200 Thiocarbonyl compounds, 280 Thioethers from carbocations, 107 Thioketones, 280 Thiols from carbocations, 107 reaction with RS.

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